From what I know, clients should be able to connect to the 5.0-1 band on your 5300 AiMesh router; and the 5.0-2 band should only be usable by a wireless AiMesh backhaul. And, clients should be able to connect to both bands on the 68U AiMesh node; otherwise, what's the point of that node if it can't extend WiFi coverage for both bands.
If you've got weird things happening, maybe you need to build it back up, one piece at a time. The 68U node should offer both bands to clients. Make sure all radios are broadcasting their signal.
OE